Thorium sounds like a good candidate. Are there lighter weight alpha emitters that might give much higher output to mass ratio for such application?. Of course it would have to be an alpha emitter with relatively long natural half life, otherwise it would be exhausted too fast for long endurance power output.
As you suggest, I suspect there's going to be a tradeoff that is made between potential thrust and how long the alpha emitter lasts. Most of the alpha emitters are heavier isotopes. Alpha decay is not an all-or-nothing thing, and if there is a way to induce activity, it's possible that some lighter elements that appear to be stable are in fact only "quasi-stable" and that activity can be induced in these under suitable conditions (this possibility is discussed in [1]).
Is there other evidence of laser stimulation of alpha decay other than say Letts / Hagelstein?... it is a fascinating idea to me.
The Letts-Hagelstein paper is one of a number of experiments that lend themselves to an interpretation of "LENR-as-induced-decay." Think of any LENR experiment that shows a correlation between helium and heat, for example. Nonetheless I am open to there being several different things going on in LENR, all of which have escaped scientific scrutiny up to now, just because of the controversy surrounding the subject.